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Join Date: Aug 1999
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There are lots, but one that just popped immediately into my head was "Sweet Jane" by the Cowboy Junkies, used in "Natural Born Killers".
Oh, and two others, which strangely both involve Kristen Stewart:
1. "Don't Dream it's Over" which used in Adventureland
2. "Begin" by The Wailin Jennys, which is used in "The Cake Eaters", a woefully under-appreciated movie. The point at which that song comes in is so perfect, it brings me to tears every time.